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Separation of Chiral Compounds

The following is a list revised from the article Optical Isomer Separation by liquid Chromatography, by Daniel Armstrong, Analytical Chemistry, Vol. 59, No. 2, Jan., 15, 1987.


Examples of Commercially Available Chiral Stationary Phases



Chiral Phase Type               Type Mobile Phase Used          Compounds Separated


¼-complex-hydrogen bonds


(R)- or (S)-N-(3,5-dinitro-     Normal Phase                    Aromatic Sulfoxides;

benzoyl)phenylglycine;          (hexane-isopropanol)            3,5 dinitrobenzoyl derivatives

ionically or covalently bonded                                  of amines, alcohols, thiols,

                                                                amino acids, amino alcohols,

                                                                hydroxy acids; aryl-substituted

                                                                lactams, succinamides,

                                                                hydantoins,

                                                                hydroxylphosphonates;

                                                                oxazolidones, binaphthols

                                                                

(S)-N-(3,5-dinitro-             Normal Phase                    Same as above

benzoyl)leucine; ionically      (hexane-isopropanol)            

or covalently bonded                                            


(R)-or (S)-N-(2-naphthyl)       Normal Phase                    Very high selectivities for a

analine                         (hexane-isopropanol)            variety of dinitrobenzoyl

                                                                derivatized compounds


(S)-1-(a-naphthyl)ethylamine    Normal Phase                    3,5 dinitrobenzoyl derivatives

                                (hexane-isopropanol)            of amino acids; 3,5 dinitro-

                                                                anilide derivatives of car-

                                                                boxylic acids


(R)-, (R)-or (S)-, or (S)-a-    Normal Phase                    3,5 dinitrobenzoyl drivatives

naphthylethylaminocar-          (hexane-isopropanol)            of amines, amides, amino

bonylvaline.  Several other                                     acid esters, and fungicides;

analogous CSPs based on                                         3,5 dinitroanilide derivatives

different amino derivatives                                     of carboxylic acids; other

are offered                                                     derivatives of the above

                                                                compounds


Cyclodextrins


b-Cyclodextrin                  Reversed Phase                  Dansyl and naphthyl amino

                                (aqueous buffers with           acids, several aromatic drugs,

                                acetonitrile or methanol)       steroids, alkaloids, metal-

                                                                locenes, binaphthyl crown

                                                                ethers, aromatic acids,

                                                                aromatic amines, aromatic

                                                                sulfoxides



a-Cyclodextrin                  Reversed Phase                  Barbituates and other

                                (aqueous buffers with           drugs, aromatic amino acids

                                acetonitrile or methanol)


g-Cyclodextrins                 Reversed Phase                  Sterioisomers of polycyclic

                                (aqueous buffers with           aromatic hydrocarbons

                                acetonitrile or methanol)


Acetylated-b-Cyclodextrins      Reversed Phase                  Steriods, polycyclic com-

                                (aqueous buffers with           pounds

                                acetonitrile or methanol)


Chiral Polymers


Bovine Serum Albumin            Aqueous Buffers                 N-aroyl amino acids, aromatic

                                                                sulfoxides


a-Acid glycoprotein             Aqueous Buffers                 Wide variety of aromatic and

                                                                cyclic drugs


Cellulose esters (acetate,      Normal Phase                    Sulfoxide derivatives of

benzoate, cinnamate),           (hexane-isopropanol)            organophosphorus com-

phenylcarbamate                                                 pounds and insecticides,

                                                                barbiturates, cyclic thioamides,

                                                                disubstituted cyclic racemates


Cellulose tribenzyl ether       Normal Phase or alcohols        Same as above


(+)-Poly(triphenylmethyl        Methanol                        Binaphthanlene derivatives,

methacrylate)                                                   cyclic insecticides, trans-disub-

                                                                stituted racemates, bis-azulenes,

                                                                derivatized glucitol


(+)-Poly(2-pyridyl-             Methanol                        Analogous to above with

diphenylmethyl methacrylate                                     somewhat different selectivities


Ligand Exchange


Hydroxyproline                  Aqueous Buffer-Cu2+             Underivatized and some

                                                                derivatized amino acids


Amino Acid (two types)          Aqueous Buffer-Cu2+             Underivatized and some

                                                                derivatized amino acids

                                                        

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